Eyewitnesses say the armed men were "highly organised"
Russia's Foreign Minister Sergei Lavrov says any armed action by Ukrainian authorities in the east of Ukraine could undermine forthcoming talks.
He made the comments after pro-Russian militants stormed a police headquarters in the eastern Ukrainian city of Kramatorsk on Sunday.
The US has condemned Russia's role in "inciting" trouble in eastern Ukraine.
Four-party talks involving Ukraine, Russia, the US and the EU are due to start in Geneva on Thursday.
Mr Lavrov said Ukraine was "demonstrating its inability to take responsibility for the fate of the country".
Russia has so far denied that it is directly responsible for the unrest in eastern Ukraine.
But the US says there has been a "concerted campaign" by forces with Russian support to undermine the authorities in Kiev.
In a phone call, US Secretary of State John Kerry urged his Russian counterpart to de-escalate the situation or face additional consequences.
He said the raids were similar to those which preceded the Russian annexation of Crimea earlier this year.
"If Russia does not take steps to de-escalate in eastern Ukraine and move its troops back from Ukraine's border, there will be additional consequences" he warned.
It has also been announced that US Vice President Joe Biden is to travel to Ukraine in 10 days' time.
Rising tension
Heavy gunfire was heard as dozens of armed men stormed the police headquarters in Kramatorsk on Saturday.
They were reported to have arrived in buses on Saturday afternoon and to have used automatic weapons to overwhelm defenders.
Several other official buildings were also reported to have been seized in the Donetsk region on Saturday.
Militants took over official buildings in the towns of Sloviansk and Druzhkovka.
They also continued their occupation of the main administrative building in the regional capital Donetsk, which they have held for one week.
Eastern Ukraine has a large Russian-speaking population and has seen a series of protests since the ousting of Ukraine's pro-Russian President Viktor Yanukovych in February.
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